Physikalisches Kolloquium: Optical Spectroscopy of Surfaces, Thin Films and Nanostructures
Wann
Dienstag, 15. Mai 2018
15:15 bis 16:45 Uhr
Wo
R 513
Veranstaltet von
Prof. Elke Scheer und Prof. Paul Leiderer, Universität Konstanz
Vortragende Person/Vortragende Personen:
Prof. Dr. Peter Zeppelfeld, Johannes Kepler University Linz, Austria
Conceptually very simple optical methods, namely Reflectance Difference Spectroscopy (RDS/RAS) and Differential Reflectance Spectroscopy (DRS), can provide valuable insight into the structure and growth of ultrathin films in straight correlation with their electronic, optical and other physical or chemical properties. Notably, these differential optical spectroscopies can achieve sub-monolayer sensitivity and are capable of monitoring kinetic processes on surfaces in real time. This will be illustrated in selected examples dealing with the fabrication and optical characterization of functional layers, such as reconstructed surfaces [1], graphene nanoribbons [2] and ultrathin molecular films [3,4]. While the spatial resolution in the UV-VIS range is naturally limited, microscopic information on the structure and electronic properties can be obtained from complementary surface science techniques such as STM and Photoemission Electron Microscopy (PEEM). As an outlook, I will describe how optical spectroscopy and PEEM can be combined into a single experiment, thus enabling truly parallel optical spectroscopy and photoelectron microscopy at a local scale [5,6].
[1] L.D. Sun, M. Hohage, P. Zeppenfeld, Phys. Rev. B 69, 045407 (2004)
[2] R. Denk et al., Nat. Commun. 5, 4253 (2014) and Nanoscale 9, 18326 (2017)
[3] L.D. Sun, J. Gall, G. Weidlinger, C.Y. Liu, M. Denk, P. Zeppenfeld, Phys. Rev. Lett. 110, 106101 (2013)
[4] J. Gall, L. Zhang, X. Fu, P. Zeppenfeld, L. D. Sun, Phys. Rev. B 96, 125424 (2017)
[5] E. Ghanbari, Th. Wagner, P. Zeppenfeld, J. Phys. Chem. C 119, 24174 (2015)
[6] A. Navarro Quezada, M. Aiglinger, E. Ghanbari, Th. Wagner, P. Zeppenfeld, Rev. Sci. Instrum. 86, 113108 (2015)